4.4 Article

Ultrafast Vibrational Dynamics of a Charged Aqueous Interface by Femtosecond Time-Resolved Heterodyne-Detected Vibrational Sum Frequency Generation

Journal

BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN
Volume 85, Issue 7, Pages 758-760

Publisher

CHEMICAL SOC JAPAN
DOI: 10.1246/bcsj.20120051

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Funding

  1. MEXT [19056009]
  2. JSPS [22655009]
  3. FPR Program of RIKEN
  4. Grants-in-Aid for Scientific Research [22655009, 19056009] Funding Source: KAKEN

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Newly developed time-, frequency-, and phase-resolved heterodyne-detected vibrational sum frequency generation (TR-HD-VSFG) spectroscopy opens a new door to explore ultrafast vibrational dynamics of interfacial water. Here, we present the first observation of TR-HD-VSFG spectra of water at a charged monolayer/aqueous solution interface.

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