Journal
SMALL METHODS
Volume 2, Issue 5, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/smtd.201700316
Keywords
hybrid halide perovskites; materials by design; photovoltaic absorbers; solar cells
Funding
- National Natural Science Foundation of China [61722403, 11674121, 11774365]
- National Key Research and Development Program of China [2016YFB0201204]
- Recruitment Program of Global Youth Experts in China
- Program for JLU Science and Technology Innovative Research Team
- Special Fund for Talent Exploitation in Jilin Province of China
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Solar-cell materials with a tetrahedral diamond structure and its derived structures (i.e., zinc blende and chalcopyrite) are the most successful family of materials, with power conversion efficiencies exceeding 20%. Recent break-throughs based on lead halide perovskites have inspired intensive research on low-cost photovoltaics beyond diamond-structured materials. While research has focused on addressing the key challenges faced by lead halide perovskites, that is, the stability and toxicity issues, it is of greater interest to develop perovskites into a new family of solar-cell materials. Here, the recent efforts toward this goal are reviewed. The focus is on computational materials design, including single, double, 2D, and nonhalide perovskites and perovskite-like materials. Meanwhile, related experiments are also reviewed with a hope that such this will help identify potential issues as well as enlightening ideas to achieve further computation-driven materials discovery.
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