Journal
CHEMICAL COMMUNICATIONS
Volume 54, Issue 86, Pages 12258-12261Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cc06819d
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Funding
- National Natural Science Foundation of China [21572139, 21732005]
- National Science and Technology Major Projects for Major New Drugs Innovation and Development [2018ZX09711003-015]
- Fundamental Research Funds for the Central Universities [2012017yjsy103]
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A strategy for synthesizing the highly oxidized bicyclo[3.2.1]octane CD rings of aconitine is reported. The key features of the synthesis include a ring-closing metathesis to form the C-ring as well as the application of a ruthenium-catalysed enyne cycloisomerization to assemble the bridged CD ring system of aconitine.
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