Journal
CHEMICAL COMMUNICATIONS
Volume 54, Issue 91, Pages 12875-12878Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cc07444e
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Funding
- EPSRC [EP/I038748/1, EP/I019693/1, EP/K014706/1, EP/K014668/1, EP/K014854/1, EP/K014714/1, EP/M013219/1, EP/L000202]
- EPSRC [EP/K005030/1, EP/K014706/2] Funding Source: UKRI
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At high loading, methanol reacts under ambient conditions with acidic hydroxyls of H-ZSM-5 to methoxylate framework oxygen; while a significant proportion remains hydrogen bonded to the framework with a protonated geometry. The findings not only explain the data which have been published so far, but also pave a way forward for potential unravelling of the initial reaction steps in the relevant chemical processes.
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