Journal
ADVANCED MATERIALS
Volume 30, Issue 5, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201703646
Keywords
covalent organic frameworks; electrocatalysts; energy conversion; energy storage
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Funding
- Air Forces MURI program [FA9550-12-1-0037]
- National Science Foundation [NSF-CMMI-1363123, 1662288]
- open program of State Key Laboratory of Organic-Inorganic Composites at BUCT [oic-201701001]
- [buctylkxj02]
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Covalent organic frameworks (COFs) are promising for catalysis, sensing, gas storage, adsorption, optoelectricity, etc. owning to the unprecedented combination of large surface area, high crystallinity, tunable pore size, and unique molecular architecture. Although COFs are in their initial research stage, progress has been made in the design and synthesis of COF-based electrocatalysis for the oxygen reduction reaction, oxygen evolution reaction, hydrogen evolution reaction, and CO2 reduction in energy conversion and fuel generation. Design principles are also established for some of the COF materials toward rational design and rapid screening of the best electrocatalysts for a specific application. Herein, the recent advances in the design and synthesis of COF-based catalysts for clean energy conversion and storage are presented. Future research directions and perspectives are also being discussed for the development of efficient COF-based electrocatalysts.
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