4.7 Article

Plasmonic silver loaded hybrid Bi-Ag nanoalloys for highly efficient disinfection by enhancing photothermal performance and interface capability

Journal

CHEMICAL ENGINEERING JOURNAL
Volume 450, Issue -, Pages -

Publisher

ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2022.138016

Keywords

Bi-Ag NPs; Hybrid alloy; Photothermocatalysis; Disinfection; Interface engineering

Funding

  1. Science and Technology Projects of Xiamen City [3502Z20194017]
  2. Natural Science Foundation of Fujian Province [2021J011328]
  3. National Natural Science Foundation of China [U1967211, 11975191]

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This study introduces the design of Bi-Ag nanoparticles with high antibacterial properties and great potential in bacterial capture and elimination. The nanoparticles also contribute significantly to improving photothermal conversion efficiency and photothermocatalytic activity.
Environmental pollution caused by bacterial infection poses a serious threat to human society. The emergence of high-performance antibacterial agents needs to be continuedly explored. Herein, surface plasmon resonance (SPR) silver-loaded hybrid photothermal-catalyst Bi-Ag nanoparticles (Bi-Ag NPs) were designed to solve the bacterial problems. The Bi-Ag NPs can effectively utilize their advantages to maximize the use of light energy. Meanwhile, the localized surface plasmon resonance and hybrid structure can be employed as a thermal reflector that not only relieves effectively the recombination of photonic electrons to promote photothermocatalytic ac-tivity but also the photothermal conversion efficiency was expanded to nearly 1.5 times compared to the single Bi NPs. Interestingly, the hybrid Bi-Ag NPs exhibit greatly fascinating ability in the bacterial capture, which is more conducive to the elimination of bacteria owing to the strong photoactivation effect at a high contact interface between bacteria and the Bi-Ag NPs. The synthesized Bi-Ag NPs performed the photothermal-catalytic anti-bacterial and purification, and further provided an inspired insight for the investigation of photothermal-catalytic nanomaterials in environmental fields.

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