Journal
PHYSICAL REVIEW B
Volume 61, Issue 6, Pages R3826-R3829Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.61.R3826
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We report on the magnetic resonance of NH3K3C60 powders in the frequency range 9-225 GHz. The observation of an antiferromagnetic resonance below the phase transition at 40 K is evidence for an antiferromagnetically ordered ground state. In the normal state, above 40 K, the temperature dependence of the spin susceptibilty measured by electron-spin resonance agrees with previous static measurements and is too weak to be explained by interacting localized spins in an insulator. The magnetic-resonance linewidth has an unusual magnetic-field dependence which is large and temperature independent in the magnetically ordered state and decreases rapidly above the transition. These observations agree with the suggestion that NH3K3C60 is a metal in the normal state and undergoes a Mott-Hubbard metal to insulator transition at 40 K.
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