Journal
TETRAHEDRON LETTERS
Volume 41, Issue 12, Pages 1907-1911Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/S0040-4039(00)00058-7
Keywords
oxidative phenolic coupling; peroxidase; cross-coupling reactions; vancomycin; biotransformations
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The bis-diaryl ether cross-linked amino acid fragment, which constitutes the upper part of a vancomycin aglycone framework, was synthesized for the first time using an enzymatic oxidative phenolic coupling methodology. This was achieved via two peroxidase-catalyzed reactions of three amino acid derivatives, 2, 3a, and 4. Other C-O and C-C hetero and homo coupling products were also obtained. (C) 2000 Elsevier Science Ltd. All rights reserved.
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