Journal
PHYSICAL REVIEW LETTERS
Volume 84, Issue 14, Pages 3181-3184Publisher
AMERICAN PHYSICAL SOC
DOI: 10.1103/PhysRevLett.84.3181
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We report a dynamical study on the photoinduced cooperative changes of the spin configurations in single crystals of the organometal spin-crossover complex. In the photoswitching process between low- and high-spin states, nonlinear characteristics such as thresholdlike behavior, incubation period, and phase separation have been observed. These results demonstrate that the cooperative intersystem crossing mediated by spin-lattice interaction plays a key role in the driving process of a new class of nonequilibrium phenomena so called photoinduced phase transition.
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