Journal
ORGANIC LETTERS
Volume 2, Issue 10, Pages 1379-1381Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol005676d
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A new silyl group, the benzhydryldimethylsilyl group, has been developed that is easily synthesized and that undergoes facile oxidation. The [3 + 2] annulation reactions of allylic silanes with this silyl group provide a variety of highly substituted five-membered carbocycles and heterocycles with high stereoselectivities. The silyl groups of these cyclic compounds have been oxidized to hydroxyl groups to demonstrate the general synthetic utility of the method.
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