Journal
PHYSICAL REVIEW LETTERS
Volume 84, Issue 23, Pages 5308-5311Publisher
AMERICAN PHYSICAL SOC
DOI: 10.1103/PhysRevLett.84.5308
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We demonstrate efficient, pulsed, gas-phase, nonlinear frequency conversion in a quadruply resonant, double-Lambda system and, simultaneously, verify theoretical predictions of Rabi-frequency matching unique to absorbing nonlinear media. This system is used to up-convert ultraviolet light at 233 nm to the vacuum ultraviolet at 186 nm in atomic Pb vapor with small-signal conversion efficiencies exceeding 30% and with modest atomic density-length (NL) products (scale 10(14) cm(-2)) and optical power densities (10-100 kW/cm(2)).
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