Journal
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA
Volume 108, Issue 1-3, Pages 89-98Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/S0368-2048(00)00148-1
Keywords
femtosecond wavepacket; photoelectron spectra; photoelectron matrix element
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Femtosecond energy- and angle-resolved pump-probe photoelectron spectra of wavepackets in a double-minimum state of Na, are studied. These studies illustrate that a robust description of the photoionization dynamics significantly enhances the utility of time-resolved photoelectron spectroscopy as a probe of wavepackets and of the evolution of electronic structure, particularly in regions of avoided crossings, and that the dependence of these angular distributions on the relative polarizations of the pump and probe lasers can be exploited to monitor molecular alignment. (C) 2000 Elsevier Science BN. All rights reserved.
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