4.8 Article

Raman generation by phased and antiphased molecular states

Journal

PHYSICAL REVIEW LETTERS
Volume 85, Issue 3, Pages 562-565

Publisher

AMERICAN PHYSICAL SOC
DOI: 10.1103/PhysRevLett.85.562

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We use molecular deuterium and two driving lasers to demonstrate collinear generation of mutually coherent equidistant sidebands, covering 50 000 cm(-1) of spectral bandwidth and ranging front 2.93 mu m to 195 nm in wavelength. The essential idea is the adiabatic preparation of a single, highly coherent (\rho(ab)\ = 0.33) molecular eigenstate.

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