Journal
NATURE
Volume 407, Issue 6800, Pages 57-60Publisher
MACMILLAN PUBLISHERS LTD
DOI: 10.1038/35024031
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The motion of electrons through quantum dots is strongly modified by single-electron charging and the quantization of energy levels(1,2). Much effort has been directed towards extending studies of electron transport to chemical nanostructures, including molecules(3-8), nanocrystals(9-13) and nanotubes(14-17). Here we report the fabrication of single-molecule transistors based on individual C-60 molecules connected to gold electrodes. We perform transport measurements that provide evidence for a coupling between the centre-of-mass motion of the C-60 molecules and single-electron hopping(18)-a conduction mechanism that has not been observed previously in quantum dot studies. The coupling is manifest as quantized nano-mechanical oscillations of the C-60 molecule against the gold surface, with a frequency of about 1.2 THz. This value is in good agreement with a simple theoretical estimate based on van der Waals and electrostatic interactions between C-60 molecules and gold electrodes.
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