Journal
PHYSICAL REVIEW B
Volume 62, Issue 14, Pages R9223-R9227Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.62.R9223
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Inelastic x-ray scattering from oxygen Is electrons in liquid and solid water were recorded up to 200 eV above the onset of the O K edge. The-partial radial distribution function that characterizes the local environment of oxygen in the water/ice system was determined. Good agreement is found between the resulting partial distribution function for liquid water and that obtained from elastic neutron scattering. In the near-edge region distinct differences between the solid and liquid states are observed which arise form differences in the local structural and electronic environment of the oxygen atoms. The method thus promises a degree of insight into details of hydrogen bonding interactions.
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