Journal
JOURNAL OF PHYSICAL CHEMISTRY A
Volume 104, Issue 40, Pages 9136-9143Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jp001157g
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The propagation of arsenous acid-iodate reaction fronts of different net stoichiometries in externally applied de electric fields is studied for a range of both electric field intensities and initial compositions of the reacting mixture (represented by the stoichiometric factor S-0). Regions of three different types of net stoichiometry in the parametric space E/V vs S-0, where E is the intensity of the applied electric field and V the reaction front propagation Velocity, are determined both experimentally and by analyzing a reaction-diffusion-migration model that includes a realistic kinetic scheme of the reaction studied. Both agreement with and discrepancies between the theoretical predictions and experimental findings are discussed.
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