Journal
GEOCHIMICA ET COSMOCHIMICA ACTA
Volume 64, Issue 22, Pages 3913-3922Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/S0016-7037(00)00488-9
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The Al-26-Mg-26 systems of five ferromagnesian chondrules from the least metamorphosed ordinary chondrite Semarkona (LL3.0) were studied using a secondary ion mass spectrometer. Their glass or plagioclase portions contain excesses of Mg-26, and in two chondrules the Mg-26 excesses are well correlated with Al-27/Mg-24, which demonstrates the in-situ decay of Al-26. The initial Al-26/Al-27 ratios in these chondrules obtained from the slope of isochrons show a narrow range of between 6 X 10(-6) and 9 X 10(-6), indicating their short formation duration of less than 1 My. If the solar nebula was initially homogeneous in Al isotopes, the chondrule formation ages are similar to2 My younger than those of CAIs. Our results based on the study of the least metamorphosed UOC are consistent with the previous studies on Al-rich chondrules that the chondrule formation started at least 2 My after CAIs. Alternatively, the older records before 2 My were erased by chondrule recycling process. It further suggests that the young apparent ages (3 to >5 My after CATs) for chondrules in type 3.4 UOCs are due to the disturbance of the Al-26-Mg-26 system, possibly during parent body metamorphism. The result is not consistent with the extended nebular time scale of >5 My and the chondrule formation by planetary processes. The Ni isotopic analysis of the FeO-rich olivines in a type IT chondrule in Semarkona did not show any detectable excess Ni-60 in spite of their high Fe/Ni ratios. The upper limit of the initial Fe-60/Fe-56 ratio of the solar system was estimated to be 3.4 x 10(-7), which is consistent with the previous estimate (0.2-1.9 X 10(-7)) from eucrites. This result confirms that the 60Ni excess previously observed from CATs was not due to the decay of the short-lived nuclide Fe-60, but a Ni isotopic anomaly of nucleosynthetic origin. Copyright (C) 2000 Elsevier Science Ltd.
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