Journal
INORGANIC CHEMISTRY
Volume 39, Issue 23, Pages 5176-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ic0005285
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The novel title compound {(Ni4Mo12v)-Mo-II} demonstrates the concept of generating targeted spin topologies using reduced polyoxometalates: The four electrophilic nickel centers-forming a tetrahedron-are fixed by a nucleophilic highly reduced diamagnetic epsilon -Keggin cluster of T-d symmetry generated in solution. This cluster not only has a structural role but actually participates in the transmission of the exchange interaction.
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