Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 113, Issue 22, Pages 9889-9892Publisher
AMER INST PHYSICS
DOI: 10.1063/1.1330235
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A hydrogen-bonded complex of OH with CO is identified along the reaction coordinate for the OH+CO <----> HOCO -->H+CO2 reaction. The existence of this linear OH-CO complex is established by infrared action spectroscopy, which accesses vibrational stretching and bending modes of the complex. Complementary electronic structure calculations characterize the OH-CO and OH-OC complexes, the transition state for HOCO formation, and the reaction pathways that connect these complexes directly to the HOCO intermediate. (C) 2000 American Institute of Physics. [S0021-9606(00)02246-7].
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