4.8 Article

Saddles in the energy landscape probed by supercooled liquids

Journal

PHYSICAL REVIEW LETTERS
Volume 85, Issue 25, Pages 5356-5359

Publisher

AMERICAN PHYSICAL SOC
DOI: 10.1103/PhysRevLett.85.5356

Keywords

-

Ask authors/readers for more resources

We numerically investigate the supercooled dynamics of two simple model liquids exploiting the partition of the multidimensional configuration space in basins of attraction of the stationary points (inherent saddles) of the potential energy surface. We find that the inherent saddle order and potential energy are well-defined functions of the temperature T. Moreover, by decreasing T, the saddle order vanishes at the same temperature (T-MCT) where the inverse diffusivity appears to diverge as a power law. This allows a topological interpretation of T-MCT: it marks the transition from a dynamics between basins of saddles (T > T-MCT) to a dynamics between basins of minima (T < T-MCT).

Authors

I am an author on this paper
Click your name to claim this paper and add it to your profile.

Reviews

Primary Rating

4.8
Not enough ratings

Secondary Ratings

Novelty
-
Significance
-
Scientific rigor
-
Rate this paper

Recommended

No Data Available
No Data Available