Journal
CHEMICAL PHYSICS LETTERS
Volume 335, Issue 1-2, Pages 27-33Publisher
ELSEVIER
DOI: 10.1016/S0009-2614(01)00005-7
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Femtosecond pump-probe spectroscopy was used to directly monitor, in the time domain, energy transfer from the blue-emitting poly(9,9-dioctylfluorene) conjugated polymer to the red-emitting tetraphenylporphyrin molecule. This system is under investigation for use as saturated red light-emitting component in an organic full-color display. The differential transmission spectrum of the system evolves, within a few picoseconds after photoexcitation, from that of the host polymer to that of the guest molecule. Experiments performed at different acceptor concentrations provide clear evidence for a Forster energy transfer mechanism and allow a determination of the interaction radius. A value of 4.2 +/- 0.2 nm was found. (C) 2001 Elsevier Science B.V. All rights reserved.
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