Journal
SURFACE SCIENCE
Volume 474, Issue 1-3, Pages L213-L216Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/S0039-6028(00)01056-6
Keywords
catalysis; vanadium oxide; titanium oxide; oxidation; alcohols
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Submonolayer to multi-layer quantities of vanadia in the +5 oxidation state were successfully prepared on TiO2(1 1 0) by codosing VOCl3 and water vapor. This vanadia selectively oxidizes methanol to formaldehyde with concomitant reduction of the vanadium cation to V3+. Reoxidation to V5+ is easily accomplished by reaction with dioxygen. (C) 2001 Elsevier Science B.V. All rights reserved.
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