Journal
PHYSICAL REVIEW A
Volume 64, Issue 2, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.64.022903
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The rotational eigenvalues of isotopically substituted hydrogen molecules adsorbed into single-walled carbon nanotubes are calculated using a semiclassical method and using a model potential. The resulting eigenvalues are used to calculate the separation factors due to rotational confinement between different isotopic species as a function of temperature and nanotube size. The results show that even for small shifts in the eigenvalues, significant fractionations should occur, suggesting possible application as an isotope-separation technique.
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