Journal
BEILSTEIN JOURNAL OF ORGANIC CHEMISTRY
Volume 10, Issue -, Pages 276-281Publisher
BEILSTEIN-INSTITUT
DOI: 10.3762/bjoc.10.23
Keywords
abietane; absolute configuration; Ceriops decandra; circular dichroism; decandrinin; Rhizophoraceae
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Funding
- NSFC [31100258, 31170331, 81125022]
- Guangdong Key Science and Technology Special Project [2011A080403020]
- Special Financial Fund of Innovative Development of Marine Economic Demonstration Project [GD2012-D01-001]
- BEBUC Excellence Scholarship System
- Else-Kroner-Fresenius-Stiftung
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Decandrinin (1), an unprecedented C-9-spiro-fused 7,8-seco-ent-abietane, was obtained from the bark of an Indian mangrove, Ceriops decandra, collected in the estuary of Godavari, Andhra Pradesh. The constitution and the relative configuration of 1 were determined by HRMS (ESI) and extensive NMR investigations, and the absolute configuration by circular dichroism (CD) and optical-rotatory dispersion (ORD) spectroscopy in combination with quantum-chemical calculations. Decandrinin is the first 7,8-seco-ent-abietane.
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