Journal
JOURNAL OF ALLOYS AND COMPOUNDS
Volume 327, Issue 1-2, Pages 253-262Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/S0925-8388(01)01465-7
Keywords
thermodynamic assessment; silica; phase diagram; volumetric properties
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Taking into account various available experimental data, an improved internally consistent data set for the SiO2 system is obtained by thermodynamic assessment. The volumetric properties for SiO2 polymorphs are reassessed using the CALPHAD method. A two-coefficient expression is used to describe the thermal expansion and bulk modulus. For liquid phase, one equation is achieved in the temperature range of 298-4000 K either for thermal expansion or for bulk modulus. Phase diagrams have been calculated up to 40 GPa. It has been concluded that, in the pressure range lower than 20 GPa, there is no significant difference between the phase diagrams calculated by the Birch-Murnaghan equation of state (EOS) and by Murnaghan EOS. (C) 2001 Elsevier Science B.V. All rights reserved.
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