Journal
CHEMICAL PHYSICS LETTERS
Volume 345, Issue 1-2, Pages 72-80Publisher
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DOI: 10.1016/S0009-2614(01)00865-X
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The femtosecond photodynamics of CF3I were studied employing the velocity mapping ion imaging technique. The angular and velocity distributions of I+ fragments were obtained as a function of the time delay between a femtosecond pump pulse at 264 nm and a probe pulse at 396 nm. The images reveal a dependence of the three-dimensional recoil distributions on the pump-probe delay time and the mutual polarization direction of pump and probe pulses. The ion velocity images provide information on the competition of different multi-photon pathways producing the ionic fragments. (C) 2001 Elsevier Science B.V. All rights reserved.
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