Journal
APPLIED CATALYSIS A-GENERAL
Volume 224, Issue 1-2, Pages 201-207Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/S0926-860X(01)00820-1
Keywords
gas phase; partial oxidation; methane; methanol
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Gas phase partial oxidation of methane to methanol has been carried out in a specially designed reactor. A comparatively high yield of methanol (ca. 7-8%, methanol selectivity of 60% at methane conversion 13%) was obtained over a quite wide temperature range of more than 40degreesC at 5.0 MPa and CH4/O-2/N-2 = 100/10/10 (ml/min). The effects of the total flow rate, CH4/O-2 ratio and pressure were examined and the superiority of the new reactor is discussed. (C) 2002 Elsevier Science B.V. All rights reserved.
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