Journal
PHYSICAL REVIEW LETTERS
Volume 88, Issue 16, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.88.160402
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We study the photodissociation chemistry of a quantum degenerate gas of bosonic triatomic ABC molecules, assuming two open rearrangement channels (AB + C or A + BC ). The equations of motion are equivalent to those of a parametric multimode laser, resulting in an exponential buildup of macroscopic mode populations. By exponentially amplifying a small differential in the single-particle rate coefficients, Bose stimulation leads to a nearly complete selectivity of the collective N -body process, indicating a novel type of ultraselective quantum degenerate chemistry.
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