Journal
OPTICS LETTERS
Volume 27, Issue 13, Pages 1168-1170Publisher
OPTICAL SOC AMER
DOI: 10.1364/OL.27.001168
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We demonstrate a significant improvement in signal-to-noise ratio in coherent anti-Stokes Raman scattering (CARS) spectroscopy/microscopy, using two highly synchronized picosecond Ti:sapphire lasers. A temporal jitter between the pulse trains from the two independent commercial lasers is reduced from a few picoseconds to similar to21 fs. maintained over several hours. The tight synchronization brings the fluctuation of the CARS signal down to the shot-noise limit. leading to enhanced CARS vibrational images of living cells and polymer beads. (C) 2002 Optical Society of America.
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