Journal
PHYSICAL REVIEW LETTERS
Volume 89, Issue 4, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.89.043001
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Nonlinear x-ray four-wave mixing experiments are becoming feasible due to rapid advances in high harmonic generation and synchrotron radiation coherent x-ray sources. By tuning the difference of two x-ray frequencies across the valence excitations, it is possible to probe the entire manifold of molecular electronic excitations. We show that the wave vector and frequency profiles of this x-ray analogue of coherent Raman spectroscopy provide an excellent real-space probe that carries most valuable structural and dynamical information, not available from spontaneous Raman techniques.
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