Journal
ACCOUNTS OF CHEMICAL RESEARCH
Volume 35, Issue 9, Pages 695-705Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ar010068z
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An important first step in making organic reactions more environmentally benign by design requires processes that are, to a first approximation, simple additions with anything else needed only catalytically. Since so few of the existing reactions are additions, synthesis of complex molecules requires the development of new atom-economic methodology. The prospect for such developments is probed in the context of ruthenium-catalyzed reaction's. Using mechanistic reasoning; over 20 new processes of varying complexity have been designed and implemented. While. some involved oxidation-reduction processes, most involved C-C bond-forming reactions.
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