Journal
PHYSICAL REVIEW LETTERS
Volume 89, Issue 20, Pages -Publisher
AMERICAN PHYSICAL SOC
DOI: 10.1103/PhysRevLett.89.203003
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Perturbative chirped pulse excitation leads to oscillations of the excited state amplitude. These coherent transients are governed by interferences between resonant and off-resonant contributions. Control mechanisms in both frequency and time domain are used to modify these dynamics. First, by applying a phase step in the spectrum, we manipulate the phase of the oscillations. By direct analogy with Fresnel zone lenses, we then conceive highly phase-amplitude modulated pulse shapes that slice destructive interferences out of the excitation time structure and enhance the final population.
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