Journal
JOURNAL OF PHYSICAL CHEMISTRY A
Volume 106, Issue 45, Pages 10843-10848Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jp020535+
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Photodissociation dynamics of SO2 were investigated employing a multiphoton pump-probe excitation technique (312 nm pump/624 nm probe), with evidence supporting the processes being initiated through the (E) over tilde state. The pump-probe optical transient for the SO2 species was fit to a single-exponential decay, yielding a time of 271 +/- 8 fs. Subsequent decay products of SO and S were also investigated and mathematically fit to determine formation and/or decay time dynamics.
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