Journal
PHYSICAL REVIEW B
Volume 66, Issue 20, Pages -Publisher
AMERICAN PHYSICAL SOC
DOI: 10.1103/PhysRevB.66.205110
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We present systematic conceptual and experimental investigations of the bulk contribution to surface sum-frequency generation (SFG) from an isotropic medium. A practical method for the analysis of spectra obtained in a transmission geometry is presented which allows to estimate the bulk contribution in any future application. A systematic degeneracy due to the molecular nature of the material is found which makes a subtle interpretation of transmission experiments necessary. Practical consequences for the analysis of typical SFG spectra are discussed.
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