Journal
PHYSICAL REVIEW LETTERS
Volume 89, Issue 27, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.89.275503
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The hole-vibrational coupling is reported for anthracene, tetracene, and pentacene on the basis of a joint experimental and theoretical study of ionization spectra using high-resolution gas-phase photoelectron spectroscopy and first-principles correlated quantum-mechanical calculations. The hole-vibrational coupling is found to be significantly smaller than the electron-vibrational coupling in the case of these oligomers; however, both quantities are predicted to converge to the same value when increasing the chain length.
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