Journal
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
Volume 2003, Issue 3, Pages 499-506Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.200390086
Keywords
aminopropenones; density functional calculations; hydrogen bonds; self-assembly
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Because of the electron-donating effects of their terminal dimethylamino groups, the carbonyl units of 1-aryl-3-(dimethylamino)prop-2-en-1-ones are excellent proton acceptors. Intra- and intermolecular hydrogen bonds formed by these species were investigated by structural techniques (Xray and neutron diffraction), spectroscopy, and density functional calculations. Co-crystallization of a derivative bearing three (dimethylamino)prop-2-en-1-one units attached at one center in the presence of different proton donors produced one- and two-dimensional H-bridged polymers. ((C) Wiley-VCH Verlag GmbH & Co. KGaA, 69451 Weinheim, Germany, 2003).
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