4.6 Article

Effect of stratosphere-troposphere exchange on the future tropospheric ozone trend

Journal

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
Volume 108, Issue D12, Pages -

Publisher

AMER GEOPHYSICAL UNION
DOI: 10.1029/2002JD002617

Keywords

stratosphere-troposphere exchange; tropospheric ozone; climate change; tropospheric chemistry; chemistry transport modeling

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[1] This paper investigates the impact of circulation changes in a changed climate on the exchange of ozone between the stratosphere and the troposphere. We have identified an increase in the net transport of ozone into the troposphere in the future climate of 37%, although a decreased ozone lifetime means that the overall tropospheric burden decreases. There are regions in the midlatitudes to high latitudes where surface ozone is predicted to increase in the spring. However, these increases are not significant. Significant ozone increases are predicted in regions of the upper troposphere. The general increase in the stratospheric contribution (O(3)s tracer) to tropospheric ozone in the climate changed scenario indicates that the stratosphere will play an even more significant role in the future.

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