Journal
APPLIED SURFACE SCIENCE
Volume 212, Issue -, Pages 349-352Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/S0169-4332(03)00100-4
Keywords
zinc oxide; nanoclusters; laser ablation; photoluminescence; laser annealing
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We present the results of experiments on synthesis of ZnO nanoclusters by reactive pulsed laser deposition (PLD). The nanoclusters were formed and crystallised in the gas phase and deposited on SiO2 substrates. The nanostructured films were characterised by conventional photoluminescence (PL). The PL spectra consist of a narrow UV excitonic band and a broad visible band related to defects in the film. The film preparation conditions such as the substrate temperature, ambient gas nature and pressure, were optimised in order to increase the intensity of excitonic emission and prevent the formation of defects. A post-growth annealing by UV laser radiation improved the optical quality of the deposited films. The photoluminescence intensity was found to be dependent significantly on the laser fluence and on the number of shots per site. The nature of the defects responsible for the observed luminescence in a visible range is discussed. (C) 2003 Elsevier Science B.V. All rights reserved.
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