Journal
CHEMICAL PHYSICS LETTERS
Volume 374, Issue 3-4, Pages 326-333Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/S0009-2614(03)00710-3
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We demonstrate the excitation of a molecular vibrational coherence via impulsive stimulated Raman scattering (ISRS) by using a pump pulse longer than the vibrational period of the excited mode. By making use of the reshaping of the pump pulse during nonlinear propagation, a Raman vibrational coherence can be excited via ISRS with a pump pulse incapable of such excitation at the input of the medium. (C) 2003 Elsevier Science B.V. All rights reserved.
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