Journal
JOURNAL OF PHYSICAL CHEMISTRY B
Volume 107, Issue 24, Pages 5857-5863Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jp030088d
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Light- and voltage-induced changes in the microwave reflectivity of semiconductors can be used to study the kinetics and mechanisms of electron transfer at semiconductor I electrolyte interfaces. The theory of the method is developed and illustrated by numerical calculations of the steady-state microwave response for low-doped silicon. The results define the range of rate constants that should be experimentally accessible using microwave reflectivity methods. The time and frequency responses of light-induced microwave reflectivity changes are considered, and it is shown that they can be used to derive values of electron transfer and recombination rate constants.
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