Journal
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
Volume 2003, Issue 14, Pages 2552-2555Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.200300196
Keywords
coordination modes; cyclization; enynes; N,P ligands; palladium
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A highly effective Cl-symmetric gem-dimethyl N,P-ligand has been developed for enantioselective palladium(II)-catalyzed carbocyclization of 1,6-enynes, in which the N/C trans mode is established for the first time in the Mizoroki-Heck-type transition state by virtue of the Cl-symmetric N,P-ligand. ((C) Wiley-VCH Verlag GmbH & Co. KGaA, 69451 Weinheim, Germany, 2003).
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