Journal
PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY OF LONDON SERIES A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES
Volume 362, Issue 1819, Pages 1239-1245Publisher
ROYAL SOC LONDON
DOI: 10.1098/rsta.2004.1376
Keywords
self-assembly; molecular recognition; combinatorial chemistry
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The principles of an evolution-selection approach to the synthesis of systems capable of molecular recognition are described. Using this dynamic combinatorial self-assembly concept in bulk solution, a variety of successful synthetic receptors have been prepared. The reversible chemistries employed include metalloporphyrin-ligand coordination, hydrazone exchange and disulfide exchange. The prospects for extension of the approach to surfaces are briefly considered.
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