Journal
ORGANIC LETTERS
Volume 6, Issue 13, Pages 2253-2256Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol049213+
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[GRAPHICS] Asymmetric reduction of ketimines 1 with trichlorosilane can be catalyzed by a new N-methyl L-valine derived Lewis basic organocatalyst, such as 4d, with high enantioselectivity. The structure-reactivity investigation suggests hydrogen bonding and arene-arene interactions between the catalyst and the incoming imine as the main factor determining the enantiofacial selectivity.
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