4.7 Article

Low-operating temperature NO2 gas sensors based on hybrid two-dimensional SnS2-reduced graphene oxide

Journal

APPLIED SURFACE SCIENCE
Volume 462, Issue -, Pages 330-336

Publisher

ELSEVIER SCIENCE BV
DOI: 10.1016/j.apsusc.2018.08.115

Keywords

2D materials; SnS2; Reduced graphene oxide (rGO); Gas sensor; Hybrid; Low operating temperature

Funding

  1. Australian Government Research Training Program Scholarship
  2. Australian Research Council - Discovery Project [ARC DP180102752]
  3. ARC [DP150101939]
  4. Queensland Government through the Q-CAS Collaborative Science Fund 2016

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The excellent sensing capabilities of SnS2 and the electrical properties of reduced graphene oxide (rGO) are combined to achieve a low-operating temperature NO2 gas sensor. Conductometric gas sensors based on hybrid films of 2D SnS2-rGO are fabricated and evaluated for humidity and different target gases including NO2, CH4, NH3, C2H5OH (ethanol), (CH3)(2)CO (acetone) at different operating temperatures ranging from 25 degrees C to 100 degrees C. The sensor shows exclusive selectivity and reversibility to NO2 as compared to the other analytes, with a low detection limit of 0.6 ppm and a response of 9.8% at 80 degrees C. The sensing mechanism of the hybrid SnS2-rGO system is described by analysing the effect of NO2 gas on the depletion region established at the interface between SnS2 and rGO layers.

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