Journal
PHYSICAL REVIEW LETTERS
Volume 93, Issue 2, Pages -Publisher
AMERICAN PHYSICAL SOC
DOI: 10.1103/PhysRevLett.93.023401
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We present a new method for the size selective structure determination of small isolated metal clusters in the gas phase. The technique is applied to cationic vanadium clusters containing 6 to 23 atoms, whose far infrared absorption spectra are measured in the 140-450 cm(-1) spectral range. The spectra are unique for each cluster size and are true fingerprints of the cluster's structure. By comparing the experimental spectra to spectra obtained from density-functional theory, the geometric cluster structure can be identified.
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