Journal
ACCOUNTS OF CHEMICAL RESEARCH
Volume 37, Issue 8, Pages 542-547Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ar030051b
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Whereas chiral Lewis acid catalysis has been intensively investigated, chiral Lewis base (nucleophilic) catalysis has been comparatively neglected. We have developed planar-chiral derivatives of 4-(dimethylamino)pyridine (DMAP), a highly versatile nucleophilic catalyst, that are effective in a diverse array of processes, including the Staudinger synthesis of beta-lactams, the acylation of silyl ketene acetals, and the kinetic resolution of amines.
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