Journal
APPLIED SPECTROSCOPY
Volume 63, Issue 1, Pages 57-65Publisher
SAGE PUBLICATIONS INC
DOI: 10.1366/000370209787169902
Keywords
Time-resolved spectroscopy; TRIR spectroscopy; Ultrafast measurement; Picosecond measurement; Nanosecond measurement; Infrared spectroscopy; IR spectroscopy; Transient; Vibrational; Crystal; Solids
Categories
Funding
- Science & Technology Facilities Council
- Centre for Molecular Structure and Dynamics Network
- Royal Society
- St Catharine's College, Cambridge
- EPSRC [EP/D072859/1, EP/D054397/1] Funding Source: UKRI
- STFC [CC/D00005X/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/D072859/1, EP/D054397/1] Funding Source: researchfish
- Science and Technology Facilities Council [CC/D00005X/1] Funding Source: researchfish
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Time-resolved infrared vibrational spectroscopy is a structurally sensitive probe of the excited-state properties of matter. The technique has found many applications in the study of molecules in dilute solution phase but has rarely been applied to crystalline samples. We report on the use of a sensitive pump-probe time-resolved infrared spectrometer and sample handling techniques for studies of the ultrafast excited-state dynamics of crystalline materials. The charge transfer excited states of crystalline metal carbonyls and the proton transfer of dihydroxyquinones are presented and compared with the solution phase.
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