4.7 Article

Transient electroosmotic flow induced by DC or AC electric fields in a curved microtube

Journal

JOURNAL OF COLLOID AND INTERFACE SCIENCE
Volume 278, Issue 2, Pages 497-507

Publisher

ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.jcis.2004.06.017

Keywords

transient; electroosmotic flow; DC or AC electric field; momentum diffusion

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This study investigates transient electroosmotic flow in a rectangular curved microtube in which the fluid is driven by the application of an external DC or AC electric field. The resultant flow-field evolutions within the microtube are simulated using the backwards-Euler time-stepping numerical method to clarify the relationship between the changes in the axial-flow velocity and the intensity of the applied electric field. When the electric field is initially applied or varies, the fluid within the double layer responds virtually immediately, and the axial velocity within the double layer tends to follow the varying intensity of the applied electric field. The greatest net charge density exists at the corners of the microtube as a result of the overlapping electrical double layers of the two walls. It results in local maximum or minimum axial velocities in the corners during increasing or decreasing applied electric field intensity in either the positive or negative direction. As the fluid within the double layer starts to move, the bulk fluid is gradually dragged into motion through the diffusion of momentum from the double layer. A finite time is required for the full momentum of the double layer to diffuse to the bulk fluid; hence, a certain phase shift between the applied electric field and the flow response is inevitable. The patterns of the axial velocity contours during the transient evolution are investigated in this study. It is found that these patterns are determined by the efficiency of momentum diffusion from the double layer to the central region of the microtube. (C) 2004 Elsevier Inc. All rights reserved.

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