Journal
APPLIED PHYSICS LETTERS
Volume 98, Issue 9, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.3562010
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Funding
- Department of Energy [DE-FG02-04ER46134]
- NSF [DMR 0819762]
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We present a hydrothermal method for growing millimeter-sized crystals of the quantum magnets with formula Cu4-xZnx(OH)(6)Cl-2: clinoatacamite (x=0), paratacamite (0.33 < x < 1) and herbertsmithite (x=1). These highly pure single crystals have been characterized by x-ray diffraction, chemical analysis, Raman spectroscopy, and magnetic susceptibility measurements. This synthesis success opens the door for detailed investigations of the magnetic ground-state properties of these compounds. (C) 2011 American Institute of Physics. [doi:10.1063/1.3562010]
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