4.6 Article

Photoelectric performance of TiO2 nanotube array photoelectrodes cosensitized with CdS/CdSe quantum dots

Journal

APPLIED PHYSICS LETTERS
Volume 96, Issue 15, Pages -

Publisher

AMER INST PHYSICS
DOI: 10.1063/1.3386525

Keywords

cadmium compounds; current density; electrochemical electrodes; II-VI semiconductors; photoelectric devices; photoelectrochemical cells; semiconductor nanotubes; semiconductor quantum dots; semiconductor thin films; short-circuit currents; solar cells; titanium compounds

Funding

  1. Ministry of Science and Technology [2006CB932401]
  2. National Science Foundation of China [60871002]

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The photoresponse of TiO2 nanotube-array films in the visible region is shown to have been significantly improved by sensitizing them with CdS and CdSe semiconductor quantum dots using a sequential chemical bath deposition method. These quantum dots served as cosensitizers, and the performance of corresponding photoelectrode was measured in a photoelectrochemical solar cell. A 13.0 mA/cm(2) short circuit current density is achieved with the TiO2/CdS/CdSe photoelectrode under AM 1.5G illuminations, which is higher than the direct sum of CdS and CdSe sensitized TiO2.

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